Establishing and Streamlining Mass Spectrometry Workflows for Elucidating Cross-links for Protein Conformational Analysis

Conference Year

2024

Abstract

Chemical crosslinking mass spectrometry (XL-MS) has emerged as a powerful tool for elucidating protein-protein interactions and structural dynamics in complex biological systems. We present a comparative analysis of two prominent software tools, Proteome Discoverer’s Xlinkx and Kojak, for the analysis of Cytochrome C cross-linked by the cleavable Disuccinimidyl Sulfoxide (DSSO). Xlinkx identified nine unique peptides and fourteen crosslinks with a minimum score cut off at 40 from cytochrome c digested with trypsin. Kojak identified significantly more peptides and crosslinks, but with much lower confidence. We visualized our data through PyMOL, mapping the distance of the three highest scoring crosslinks.

Primary Faculty Mentor Name

Ying Wai Lam

Status

Undergraduate

Student College

College of Arts and Sciences

Program/Major

Biochemistry

Primary Research Category

Life Sciences

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Establishing and Streamlining Mass Spectrometry Workflows for Elucidating Cross-links for Protein Conformational Analysis

Chemical crosslinking mass spectrometry (XL-MS) has emerged as a powerful tool for elucidating protein-protein interactions and structural dynamics in complex biological systems. We present a comparative analysis of two prominent software tools, Proteome Discoverer’s Xlinkx and Kojak, for the analysis of Cytochrome C cross-linked by the cleavable Disuccinimidyl Sulfoxide (DSSO). Xlinkx identified nine unique peptides and fourteen crosslinks with a minimum score cut off at 40 from cytochrome c digested with trypsin. Kojak identified significantly more peptides and crosslinks, but with much lower confidence. We visualized our data through PyMOL, mapping the distance of the three highest scoring crosslinks.